Record nonlinear conversion efficiency in the production of high spectral purity vacuum ultraviolet laser at 148 nm

Physics > Optics [Submitted on 17 Jun 2026] Title:Record nonlinear conversion efficiency in the production of high spectral purity vacuum ultraviolet laser at 148 nm View PDFAbstract:Coherent vacuum-ultraviolet (VUV) lasers are indispensable for precision measurement, quantum optics, and materials science. Recent high-resolution spectroscopy of the Th-229 nuclear clock transition near 148 nm highlights the urgent demand for intense, narrow-linewidth VUV lasers for advancing metrology and testing fundamental physics. However, existing VUV generation schemes typically require enhancement cavities [C. Zhang et al., Opt. Lett. 47, 5591-5594 (2022)], atomic resonances [Q. Xiao et al., Nature 650, 852-856 (2026)], or random quasi-phase-matched nonlinear crystals [V. Lal et al., Optica 12, 1971-1974 (2025)]. Here, we demonstrate a VUV frequency comb via cascaded frequency doubling of a 2400 nm Cr:ZnS comb to its 16th harmonic in nonlinear crystals. The final stage employs a bulk-grown, spatially uniform quasi-phase matched (QPM) crystal developed by IPG, combining VUV transparency, high $\chi^2$ nonlinearity, and power scalability. Using this QPM crystal we generate a VUV frequency comb with 40 $\mu$W average power (1 nW per mode at 80 MHz mode spacing) with a conversion efficiency order of magnitude higher than other known methods. These results establish a scalable route to compact VUV sources via direct frequency doubling, opening a path toward a robust continuous-wave nuclear clock laser. Current browse context: physics.optics Change to browse by: References & Citations Loading... Bibliographic and Citation Tools Bibliographic Explorer (What is the Explorer?) Connected Papers (What is Connected Papers?) Litmaps (What is Litmaps?) scite Smart Citations (What are Smart Citations?) Code, Data and Media Associated with this Article alphaXiv (What is alphaXiv?) CatalyzeX Code Finder for Papers (What is CatalyzeX?) DagsHub (What is DagsHub?) Gotit.pub (What is GotitPub?) Hugging Face (What is Huggingface?) ScienceCast (What is ScienceCast?) Demos Recommenders and Search Tools Influence Flower (What are Influence Flowers?) CORE Recommender (What is CORE?) arXivLabs: experimental projects with community collaborators arXivLabs is a framework that allows collaborators to develop and share new arXiv features directly on our website. Both individuals and organizations that work with arXivLabs have embraced and accepted our values of openness, community, excellence, and user data privacy. arXiv is committed to these values and only works with partners that adhere to them. Have an idea for a project that will add value for arXiv's community? Learn more about arXivLabs.